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• W1963623323 abstract "Atomic transport in the presence of a temperature gradient, commonly known as thermotransport or the thermomigration phenomenon, was simulated for U–Zr alloys using a phase-field model derived from irreversible thermodynamics. The free energy of the U–Zr system, a necessary ingredient for the phase-field-model, was directly incorporated from the available thermodynamic database. Kinetic parameters such as atomic mobility and heat of transport terms were obtained from experimental values reported in the literature. The model was applied to a single-phase (bcc-γ phase) alloy and to a diffusion couple consisting of two single-phase (bcc-γ phase) alloys of different compositions, both subjected to a constant temperature gradient. Constituent redistribution in the absence and presence of a compositional gradient was examined. An enrichment of Zr with a corresponding depletion of U was observed at the hot end of the initially homogeneous single-phase alloy. A similar atomic transport behavior was observed in the diffusion couple, where the magnitude and direction of the final composition gradient was dictated by the combined influence of atomic mobility and heat of transport terms." @default.
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• W1963623323 date "2011-07-01" @default.
• W1963623323 modified "2023-09-26" @default.
• W1963623323 title "Thermotransport in γ(bcc) U–Zr alloys: A phase-field model study" @default.
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• W1963623323 doi "https://doi.org/10.1016/j.jnucmat.2011.03.028" @default.
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