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- W1963648584 abstract "The velocity and absorption of sound waves are measured in liquid dichloromethane–benzene mixtures in the frequency range from 3 MHz to 6 GHz using three ultrasonic techniques, high-resolution Bragg reflection, Brillouin scattering, and pulse-echo overlap. Vibrational double relaxation is observed in every mixture studied. The higher-frequency relaxation is assigned to the lowest mode of benzene, and the lower-frequency one to all but the lowest mode of both molecules. These modes of both molecules are shown to be coupled with each other by the near-resonant intermolecular vibrational–vibrational energy transfers between the second lowest mode (704 cm−1) of dichloromethane and the modes (707, 675 cm−1) of benzene. The concentration dependence of the relaxation frequency is analyzed with the binary collision theory, and the rates of vibrational–translational energy transfer in collisions between different kinds of molecules are estimated." @default.
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- W1963648584 date "1981-01-15" @default.
- W1963648584 modified "2023-10-18" @default.
- W1963648584 title "Effect of near‐resonant energy transfer on vibrational relaxation in liquid dichloromethane–benzene mixtures" @default.
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- W1963648584 doi "https://doi.org/10.1063/1.441210" @default.
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