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• W1963649219 abstract "N-Heterocyclic carbene (NHC)-mediated ring-opening polymerization (ROP) of N-substituted N-carboxylanhydride (NR-NCA) yields cyclic poly(α-peptoid)s with controlled molecular weights (Mn = 3−30 kg mol−1) and narrow molecular weight distributions (PDI = 1.04−1.12). The reactions exhibit characteristics of a living polymerization with minimal chain transfer. This enables the facile synthesis of cyclic diblock copoly(α-peptoid)s through sequential monomer addition. The cyclic polymer architectures were verified by MALDI-TOF mass spectrometry and intrinsic viscosity measurements. Mark−Houwink−Sakurada plot analyses revealed that cyclic poly(α-peptoid)s prepared from NHC-mediated polymerizations exhibit lower intrinsic viscosities than their linear analogues prepared from primary amine-initiated polymerizations. The ratio of their intrinsic viscosities is consistent with the former being mostly cyclic." @default.
• W1963649219 created "2016-06-24" @default.
• W1963649219 creator A5036305730 @default.
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• W1963649219 date "2009-12-01" @default.
• W1963649219 modified "2023-10-16" @default.
• W1963649219 title "Cyclic Poly(α-peptoid)s and Their Block Copolymers from N-Heterocyclic Carbene-Mediated Ring-Opening Polymerizations of N-Substituted <i>N</i>-Carboxylanhydrides" @default.
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• W1963649219 doi "https://doi.org/10.1021/ja907380d" @default.
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