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- W1963673722 abstract "Magnetic properties of (DMe-DCNQI)2Cu, (DMeO-DCNQI)2Cu and (DBr-DCNQI)2Cu were investigated by 1H-NMR, ESR and magnetic susceptibility measurements. 1H-T1−1 was found to exhibit a step-like enhancement at the metal-insulator (M-I) transitions of DBr-salt at ambient pressure and of DMe- and DMeO-salts under pressure. This reflects the appearance of localized Cu2+ spins at the M-I transition. An antiferromagnetic (AF) ordering was observed in DBr- (at ambient pressure) and DMe-salts (under pressure). In both salts, 1H-NMR relaxation rates, T1−1, T2∗−1and T2−1, indicate the onset of inhomogeneous local field at the transition temperature, TN: The lineshape below TN is well explained by the assumption that the magnetic Cu2+-sites with μB form a regular three-fold lattice along the c-axis. In the DMe-salt, the pressure dependence of TN was determined. It was shown that the enhancement of static susceptibility in the metallic state of DMe-salt was due to the insulating domain induced by some stress within the sample." @default.
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- W1963673722 date "1993-03-01" @default.
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- W1963673722 title "Magnetism of DCNQI-Cu salts" @default.
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- W1963673722 doi "https://doi.org/10.1016/0379-6779(93)90411-o" @default.
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