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- W1963893353 abstract "Abstract Autothermal reforming of CH4 has been studied under both periodic and steady state conditions. The investigation was conducted over Co–NiO in a fluidised bed reactor at 873 K and 101.32 kPa. Cycle periods of 1–40 min were used whilst the cycle split, Sox (with respect to the O2-rich cycle) was varied from 0.1 to 0.9. Generally, CH4 oxidation stimulated CO formation, however, steam reforming yielded predominantly CO2 and H2. Although O2-rich cycling (Sox≥0.5) was detrimental to H2 formation, H2O-rich cycling resulted in a 15% improvement in steady state H2 formation. Theoretical as well as experimental investigations pointed to a resonant frequency of about 6.7 mHz for CH4 oxidation to produce super steady state H2 yields. By periodic operation, it is possible to tune H2/CO ratios over the range 2.5–7 for the same feed composition. Interestingly, Sox=0.1 yielded the highest ratios, whereas the lowest ratios were attained at Sox=0.9. Periodic composition cycling introduces a more flexible approach to reactor operation — H2/CO can be easily modulated by varying the cycle parameters — compared to steady state operation." @default.
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- W1963893353 date "2000-12-01" @default.
- W1963893353 modified "2023-09-26" @default.
- W1963893353 title "Influence of cycle parameters on periodically operated fluidised bed reactor for CH4 autoreforming" @default.
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- W1963893353 doi "https://doi.org/10.1016/s0920-5861(00)00497-1" @default.
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