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- W1963899178 abstract "Using site-specific soft x-ray emission and absorption spectroscopy in conjunction with site-specific x-ray photoelectron spectroscopy, we present measurements of the valence and conduction band states of NiO. Significant hybridization between the Ni and the O electronic states near the Fermi energy is observed throughout both the valence and conduction bands, in accordance with density-functional theory calculations also presented. The relationship between our emission and absorption measurements also shows direct similarities to other techniques used to measure the non-dipole-allowed $dtext{penalty1000-hskip0pt}d$ transitions within NiO, addressing questions concerning the character of the insulating band gap of this system. NiO has previously been described as a large-gap, charge-transfer insulator, while our data show the valence and conduction states at the Fermi energy to be primarily of Ni $d$--character hybridized with a small amount of O $p$--character states, suggesting a mixture of charge-transfer and Mott-Hubbard character as described by the Zaanen-Sawatzky-Allen model." @default.
- W1963899178 created "2016-06-24" @default.
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- W1963899178 date "2005-03-18" @default.
- W1963899178 modified "2023-10-02" @default.
- W1963899178 title "Character of the insulating state in NiO: A mixture of charge-transfer and Mott-Hubbard character" @default.
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- W1963899178 doi "https://doi.org/10.1103/physrevb.71.115113" @default.
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