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• W1964287234 abstract "The collision-induced pure dephasing rate constant of a pair of coherently excited eigenlevels of SO2 is measured. This represents the first measurement of a collision-induced pure dephasing constant for a molecule in gaseous phase. The pair of eigenlevels arises from the coupling of the C̃(210)716 level and an isoenergetic high vibrational level, 44877.52 cm-1 above the zero point, of the X̃ state. The pure dephasing cross sections measured for the three colliding partners He, Ar, and SO2 at the temperature 4.8 K are respectively 26, 40, and 720 Å2. All three pure dephasing cross sections are about a factor of 2 smaller than the corresponding depopulation cross sections. Comparison with the hard sphere and Lennard-Jones cross sections suggests that collision-induced dephasing involves more than hard sphere, repulsive forces." @default.
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• W1964287234 date "2003-11-14" @default.
• W1964287234 modified "2023-09-25" @default.
• W1964287234 title "Collision Induced Dephasing in Fluorescence Quantum Beat of SO2(C̃B2)" @default.
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• W1964287234 doi "https://doi.org/10.1021/jp030957z" @default.
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