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- W1964527524 abstract "In the perturbation theory studied by Barker and Henderson, an expansion is made of the free energy in terms of a strength parameter $ensuremath{lambda}$ that multiplies the attractive part of the potential. This expansion is shown here to converge very rapidly for the Lennard-Jones liquid. Taking as zeroth-order approximation the system with only repulsive forces, Barker and Henderson have shown that it can be approximated by hard spheres with a temperature-dependent diameter. We show by a direct computation that this approximation is excellent. In the spirit of the $ensuremath{lambda}$ expansion, we can write down a semiempirical equation of state which is applied with success to the Lennard-Jones fluid, argon, and xenon. It is seen that the large scale density variation characteristic of the critical point lowers the critical temperature by 6%." @default.
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- W1964527524 date "1969-06-05" @default.
- W1964527524 modified "2023-09-27" @default.
- W1964527524 title "Perturbation Theory and Equation of State for Fluids" @default.
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- W1964527524 doi "https://doi.org/10.1103/physrev.182.307" @default.
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