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- W1964538577 abstract "Second- and third-harmonic generation in single-wall carbon nanotube layers produced by low-velocity spraying was studied experimentally with the use of amplified 75 fs pulses of Cr:forsterite laser radiation within the range of pump pulse intensities up to the breakdown threshold. Harmonic-generation processes are shown to be ideally suited for the non-linear spectroscopy and structure analysis of carbon nanotubes, in many ways supplementary to Raman spectroscopy. The second- and third-harmonic yields scale as quadratic and cubic functions, respectively, of the pump pulse energy up to pump intensities of 1012 W cm−2, indicating the perturbative regime of non-linear-optical interactions and suggesting a convenient calibration for the second and third harmonics employed as spectroscopic probes. Comparison of harmonic-generation data with absorption spectra of carbon-nanotube layers reveals an important role of quantum confinement effects in the non-linear coherent scattering of light from carbon nanotubes. Femtosecond pulses of Cr:forsterite laser radiation also generate the fifth optical harmonic at 251 nm in the glass substrate of carbon-nanotube samples, which can be employed for UV spectroscopy and subwavelength-resolution non-linear microscopy of carbon nanotubes. Copyright © 2003 John Wiley & Sons, Ltd." @default.
- W1964538577 created "2016-06-24" @default.
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- W1964538577 date "2003-01-01" @default.
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- W1964538577 title "Femtosecond optical harmonic generation as a non-linear spectroscopic probe for carbon nanotubes" @default.
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- W1964538577 doi "https://doi.org/10.1002/jrs.1080" @default.
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