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- W1964554874 abstract "The total dielectric response of a protein in due to different kinds of motion each of them having its own, and often very different characteristic time. This situation has been described phenomenologically in terms of a set of effective dielectric constants ϵπ operative in the corresponding time intervals. The effects of this time dependence on the reaction free energy ΔG and on the medium reorganization energy Es were considered employing the models of an infinite homogeneous dielectric and of a three-layer membrane. For the primary charge separation, the effects of the variable ϵπ on both these energies, ΔG and Es, are practically equal and opposite in sign, and hence compensate each other. As a result, the primary charge separation proves to be activationless irrelevant to the value of ϵπ. On the basis of the existing experimental data, the semiquantitative estimates of ϵπ at different times were given. With these values of ϵπ, the activation energy close to zero was calculated for the fast reactions of electron transfer from bacteriopheophytin to quinone and of recombination of the primary radical-ion pair with formation of a neutral triplet." @default.
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- W1964554874 date "1995-02-01" @default.
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- W1964554874 title "Fast electron transfers in photosynthetic reaction centre: effect of the time-evolution of dielectric response" @default.
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- W1964554874 doi "https://doi.org/10.1016/0005-2728(94)00160-7" @default.
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