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- W1964983607 abstract "Abstract Results of a thermodynamic analysis of the processes proceeding on diamond (111) faces in hydrogen-rich environments are presented. It is shown that the key role of atomic hydrogen is to inhibit hydrogen desorption and subsequent surface reconstruction which is accompanied by the formation of sp2 hybridized structures on the surfaces of growing crystals. Such structures provide a template for graphite, rather than diamond formation. Furthermore, a high concentration of atomic hydrogen promotes the formation of saturated carbon-hydrogen clusters on the diamond crystal surfaces which leads to the extension of the pre-existing diamond lattice, i.e. diamond growth. The model correctly predicts the experimentally determined proportionality between the growth rate and the concentration of atomic hydrogen as well as trends in growth rate and diamond film quality as a function of methane concentration." @default.
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- W1964983607 date "1993-02-01" @default.
- W1964983607 modified "2023-09-26" @default.
- W1964983607 title "Role of atomic hydrogen in preventing surface reconstruction and sp2 bond formation during chemical vapour deposition of diamond" @default.
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- W1964983607 doi "https://doi.org/10.1016/0925-9635(93)90140-w" @default.
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