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• W1965332602 abstract "Photodetachment cross sections are measured across the detachment threshold of Au2− between 1.90 and 2.02 eV using a tunable laser. In addition to obtaining a more accurate electron affinity for Au2 (1.9393 ± 0.0003 eV), we observe eight resonances above the detachment threshold, corresponding to excitations from the vibrational levels of the Au2− ground state (X 2Σu+) to those of a metastable excited state of Au2− (or Feshbach resonances) at an excitation energy of 1.9717 ± 0.0003 eV and a vibrational frequency of 129.1 ± 1.5 cm−1. High-resolution photoelectron spectra of Au2− are obtained using photoelectron imaging to follow the autodetachment processes by tuning the detachment laser to all the eight Feshbach resonances. We observe significant non-Franck-Condon behaviors in the resonant photoelectron spectra due to autodetachment from a given vibrational level of the Feshbach state to selective vibrational levels of the neutral final state. Using the spectroscopic data for the ground states of Au2− (X 2Σu+) and Au2 (X 1Σg+), we estimate an equilibrium bond distance of 2.53 ± 0.02 Å for the Feshbach state of Au2− by simulating the Franck-Condon factors for the resonant excitation and autodetachment processes." @default.
• W1965332602 created "2016-06-24" @default.
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• W1965332602 date "2013-11-18" @default.
• W1965332602 modified "2023-09-27" @default.
• W1965332602 title "Resonant photoelectron spectroscopy of Au2− via a Feshbach state using high-resolution photoelectron imaging" @default.
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• W1965332602 doi "https://doi.org/10.1063/1.4830408" @default.
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