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- W1965440123 abstract "Spectrokinetic studies of the gas-phase equilibrium F+O2⇌FO2 have been undertaken at six temperatures between 295 and 359 K. F atoms were produced by pulse radiolysis of Ar/F2/O2 mixtures. The yield of FO2 radicals and the rates of formation and decay were studied as a function of the oxygen concentration, and the temperature dependences of both the forward and reverse rate constants, k1 and k−1, were obtained. The equilibrium constant, Kp=k1/k−1RT, was shown to be pressure independent. The computed value of ΔS2980 = −24.917 cal/mol K, when combined with the other calculated thermodynamic variables and the measured equilibrium constants, gives ΔH2980 = −12.62±0.50 kcal/mol, ΔHf,2980(FO2)=6.24±0.50 kcal/mol and an intrinsic FO2 bond strength ΔH00=11.68±0.50 kcal/mol." @default.
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- W1965440123 date "1987-10-01" @default.
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- W1965440123 title "Spectrokinetic studies of the gas-phase equilibrium F+O2⇌FO2 between 295 and 359 K" @default.
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- W1965440123 doi "https://doi.org/10.1016/0009-2614(87)80097-0" @default.
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