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- W1965543693 abstract "Solubility studies show that trivalent f-element carbonate compounds are the predominant solids that primarily limit the soluble metal ion concentration under environmental conditions. We systematically investigated the spectroscopic characteristics of a series of solid f-element (Eu and 243Am) carbonates. Varying pH, ionic strength, and carbonate concentration results in the formation of M(OH)3, MOHCO3, M2(CO3)3·nH2O, and NaM(CO3)2·nH2O, where M=Eu(III) or Am(III). Solids were characterized by FTIR, fluorescence, and EXAFS spectroscopies that determined and confirmed the coordination environment, and by their individual X-ray diffraction powder patterns. The number of coordinated crystal waters was determined to be 2–3 for Eu2(CO3)3·nH2O and 5 for NaEu(CO3)2·nH2O using thermogravimetric/differential thermal analysis and fluorescence lifetime. We report studies of the fluorescence of Am(III) and the effect of carbonate coordination on the 5D1→7F1 transition." @default.
- W1965543693 created "2016-06-24" @default.
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- W1965543693 date "2000-05-01" @default.
- W1965543693 modified "2023-10-03" @default.
- W1965543693 title "Spectroscopic characterization of trivalent f-element (Eu, Am) solid carbonates" @default.
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- W1965543693 doi "https://doi.org/10.1016/s0925-8388(00)00665-4" @default.
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