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- W1965600348 abstract "Abstract Lead(IV) chloride solutions in CCl4, CHCl3, cyclohexane, benzene, toluene, chlorobenzene, N,N-dimethylformamide and pyridine have been irradiated with an approximately 1.5 kJ pulse of UV radiation lasting 0.5 ms. The course of the photochemical processes has been followed by measuring the loss of PbCl4, the changes of Cl2 concentration and by identification of chlorination products. In a similar way, chlorine solutions in cyclohexane and benzene have been investigated. Primary processes are discussed in detail. The most probable process in solvents that do not form complexes with PbCl4 is predissociation of the PbCl bond whereas in those forming complexes with PbCl4 electron transfer takes place: The results are compared with those obtained earlier under steady irradiation. This allows us to determine new pathways of secondary processes that are unobservable with the continuous illumination technique. The pathways include processes photoinduced by the phase of fresh finely dispersed PbCl2 crystals:" @default.
- W1965600348 created "2016-06-24" @default.
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- W1965600348 date "1979-06-01" @default.
- W1965600348 modified "2023-10-16" @default.
- W1965600348 title "Pulse photolysis of PbCl4 in non-aqueous solutions" @default.
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- W1965600348 doi "https://doi.org/10.1016/0047-2670(79)80052-0" @default.
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