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• W1965600830 abstract "Fluorescence excitation spectra of 4-(diisopropylamino)benzonitrile (DIABN) and 4-(dimethylamino)benzonitrile (DMABN) in thermal vapour and seeded jet expansions are compared. The spectrum of jet-cooled DIABN shows an intense 0–0-transition at 31751.8cm−1. The spectrum collapses at excess excitation energies above 800cm−1, indicating the presence of an efficient non-radiative decay channel. In the gas phase, fluorescence emission of DIABN occurs from the intramolecular charge transfer (ICT) state. The non-radiative decay channel, therefore, is attributed to rapid ICT in the isolated molecule. The related compounds 4-(methylamino)-3,5-dimethylbenzonitrile (MHD), 4-(azetidinyl)-3,5-dimethylbenzonitrile (M4D), and 4-(dimethylamino)-3,5-dimethylbenzonitrile (MMD) in the jet show extremely weak and structureless emission." @default.
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• W1965600830 date "2001-06-01" @default.
• W1965600830 modified "2023-10-11" @default.
• W1965600830 title "Fluorescence excitation spectra of jet-cooled 4-(diisopropylamino)benzonitrile and related compounds" @default.
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• W1965600830 doi "https://doi.org/10.1016/s0009-2614(01)00365-7" @default.
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