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• W1965625540 endingPage "3914" @default.
• W1965625540 startingPage "3907" @default.
• W1965625540 abstract "Three new dyes have been synthesized to investigate the influence of the distance between the electron acceptor and TiO2 surface on the performance of dye-sensitized solar cells (DSSCs). In these dyes, the isoquinolinium acceptor, with a −(CH2)nCOOH anchoring group, and a functionalized triphenylamine donor are separated by an oligothiophene bridge. The physical and electrochemical properties of the dyes were investigated systematically. The results prove that different numbers of −CH2– units between the isoquinolinium acceptor and the carboxyl anchoring group have a less pronounced effect on the physical and electrochemical properties of these dyes. However, when applied in DSSCs, a sharp decrease in the short-circuit current (Jsc) was observed with increasing numbers of −CH2– units. For example, the device containing the organic dye bearing three −CH2– units produced the lowest Jsc of 7.94 mA·cm–2. In contrast, the device containing the dye bearing only one −CH2– unit exhibited the highest Jsc of 13.88 mA·cm–2. The higher photocurrent obtained with the device incorporating the dye with one −CH2– unit resulted in a higher power conversion efficiency of 6.8%." @default.
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• W1965625540 date "2014-03-10" @default.
• W1965625540 modified "2023-10-18" @default.
• W1965625540 title "Effect of Different Numbers of −CH₂– Units on the Performance of Isoquinolinium Dyes" @default.
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• W1965625540 doi "https://doi.org/10.1021/am405014f" @default.
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