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- W1965634189 abstract "Abstract The segregation kinetics studies of sulphur and carbon in iron and the adsorption kinetics of oxygen on iron have been discussed, taking into account the real structure of the monocrystalline sample. The deviation of the kinetics results from the t1/2 law has been interpreted as the effect of the presence of the adsorption sites in the defects of the monocrystalline iron sample. The equilibrium between the adsorption states of sulphur, carbon and oxygen atoms in the defects and on the surface has been assumed. For sulphur and carbon atoms, the energetically more favourable adsorption sites are in the defects; however, for oxygen atoms the adsorption sites on the surface are more favourable. The free energy of the segregation of sulphur and carbon atoms from the defects to the surface has been assumed to be a linear function of the degree of filling of the adsorption sites in the defects. The calculations of the energies of iron clusters with a contaminant atom have been also considered." @default.
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- W1965634189 date "1998-05-01" @default.
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- W1965634189 title "The effect of the real crystal structure of iron on the behaviour of surface contaminants" @default.
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- W1965634189 doi "https://doi.org/10.1016/s0039-6028(97)00955-2" @default.
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