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• W1965661957 endingPage "194102" @default.
• W1965661957 startingPage "194102" @default.
• W1965661957 abstract "We present a new approach for calculating quantum time correlation functions for systems whose dynamics exhibits relevant nonadiabatic effects. The method involves partial linearization of the full quantum path-integral expression for the time correlation function written in the nonadiabatic mapping Hamiltonian formalism. Our analysis gives an algorithm which is both numerically efficient and accurate as we demonstrate in test calculations on the spin-boson model where we find results in good agreement with exact calculations. The accuracy of our new approach is comparable to that of calculations performed using other approximate methods over a relatively broad range of model parameters. However, our method converges relatively quickly when compared with most alternative schemes. These findings are very encouraging in view of the application of the new method for studying realistic nonadiabatic model problems in the condensed phase." @default.
• W1965661957 created "2016-06-24" @default.
• W1965661957 creator A5032591549 @default.
• W1965661957 creator A5086249503 @default.
• W1965661957 date "2005-05-15" @default.
• W1965661957 modified "2023-09-25" @default.
• W1965661957 title "LAND-map, a linearized approach to nonadiabatic dynamics using the mapping formalism" @default.
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• W1965661957 doi "https://doi.org/10.1063/1.1896948" @default.
• W1965661957 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/16161558" @default.
• W1965661957 hasPublicationYear "2005" @default.
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