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- W1966017072 abstract "Sum frequency generation (SFG) surface vibrational spectroscopy has been used to identify reactive surface intermediates in situ during catalytic dehydrogenation reactions of high-pressure cyclohexane (C(6)H(12)) on the Pt(111) crystal surface in the presence and absence of high-pressure hydrogen. These experiments provide the first spectroscopic evidence of cyclohexyl (C(6)H(11)) as a reactive surface intermediate during the cyclohexane catalytic conversion to benzene at high pressure in the presence of excess hydrogen. In addition, it was proposed from temperature-dependent SFG experiments that dehydrogenation of cyclohexyl is a rate-limiting step in the cyclohexane catalytic conversion to benzene." @default.
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- W1966017072 date "2003-08-15" @default.
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- W1966017072 title "Evidence for Cyclohexyl as a Reactive Surface Intermediate during High-Pressure Cyclohexane Catalytic Reactions on Pt(111) by Sum Frequency Generation Vibrational Spectroscopy" @default.
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- W1966017072 doi "https://doi.org/10.1021/ja035710u" @default.
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