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• W1966145259 abstract "The conductivity of the linear-chain molecular-metal phthalocyanatonickel(II)iodide [Ni(pc)I] remains metallic down to ensuremath{sim}30 K, goes through a weak maximum, and then levels off to a high asymptotic ($Tensuremath{rightarrow}0$) value that varies from textonehalf{} to 2 times the value at room temperature (ensuremath{sim}500 ${mathrm{ensuremath{Omega}}}^{ensuremath{-}1}$ ${mathrm{cm}}^{ensuremath{-}1}$). The full characterization of this compound, reported here, includes a thermoelectric power linearly proportional to $T$, a Pauli-like static and EPR magnetic susceptibility, and single-crystal reflectivity spectra exhibiting a plasma edge for light polarized parallel to the conducting axis. The results confirm that this compound possesses all the characteristics of molecular metal that retains a metallic band structure down to a temperature below 2 K. However, Ni(pc)I does not possess any strong interstack interactions of the type necessary to suppress a Peierls metal-nonmetal transition via an increase in the dimensionality, and should be classified as one of the most one-dimensional molecular metals studied to date. A structurally imposed weakening of the interstack Coulomb interactions, coupled with weak random potentials from structurally disordered triiodide chains, is apparently sufficient to suppress the three-dimensional transition normally associated with the tendency of an anisotropic conductor to undergo a Peierls distortion." @default.
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• W1966145259 date "1984-12-01" @default.
• W1966145259 modified "2023-09-26" @default.
• W1966145259 title "Nickel phthalocyanine iodide: A highly-one-dimensional low-temperature molecular metal" @default.
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• W1966145259 doi "https://doi.org/10.1103/physrevb.30.6269" @default.
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