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• W1966163985 abstract "The dynamical properties of ${mathrm{Tb}}^{3+}$ fluorescence in ${mathrm{TbF}}_{3}$ have been investigated above and below its ferromagnetic phase transition (${T}_{C}$=3.95 K). Near and below ${T}_{C}$ the magnetic interactions lead to splittings and shifts of the optical lines reflecting the interionic interactions and the onset of the ordered state. A dramatic (factor of 10) lengthening of the exciton decay occurs both when lowering the temperature below ${T}_{C}$ and when applying an appropriate external magnetic field along the easy axis above ${T}_{C}$. Throughout the range from 300 to 1.6 K, the experimental fluorescence decays are in agreement with a rate-equation model involving fast-diffusion energy transfer among intrinsic ions. The observed decrease in diffusion coefficient can be understood either as the result of a large reduction of the resonant energy transfer between intrinsic ions or as the result of a decrease in the trapping probability in the ferromagnetic or aligned paramagnetic phases. Either process may be understood in terms of the short-range ${mathrm{Tb}}^{3+}$-${mathrm{Tb}}^{3+}$ interactions and the properties of the ordered state." @default.
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• W1966163985 date "1987-06-01" @default.
• W1966163985 modified "2023-09-26" @default.
• W1966163985 title "Effect of magnetic order on the fluorescence dynamics ofTbF3" @default.
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• W1966163985 doi "https://doi.org/10.1103/physrevb.35.8322" @default.
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