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• W1966257083 abstract "A lattice model of the metal electrode–electrolyte interface is presented which partitions the region into a number of planar layers. In each layer statistical competition occurs between ions and solvent molecules, represented as point charges and finite length dipoles, respectively. Differential capacitance and other results are compared with those of earlier models and with experiments. Agreement with experiments requires explicit inclusion of an inner layer with solvent properties which differ from the remainder of the system. The inner layer may consist of finite-length dipoles alone, or of both dipoles and charges. The use of finite length dipoles drastically changes the high field saturation properties of the layers, as compared with models involving infinitesimal (point) dipoles. Very little dielectric saturation occurs at physically realizable fields." @default.
• W1966257083 created "2016-06-24" @default.
• W1966257083 creator A5015233198 @default.
• W1966257083 creator A5091749132 @default.
• W1966257083 date "1984-10-01" @default.
• W1966257083 modified "2023-09-26" @default.
• W1966257083 title "A lattice model for the electrical double layer using finite-length dipoles" @default.
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• W1966257083 doi "https://doi.org/10.1063/1.448028" @default.
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