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• W1966282730 endingPage "88" @default.
• W1966282730 startingPage "68" @default.
• W1966282730 abstract "The widespread precatalyst (prepared in-situ or ex-situ) (arene) RuTsDPEN advocated for highly effectual asymmetric transfer hydrogenation (ATH) reactions with 2-propanol as hydrogen donor at ambient conditions, is proven to be unstable under the strong reducing conditions prevailing in the reaction mixtures (blend of alcohol and a base such as KOH). We assert that the true catalysts are the ruthenium metal nanoclusters formed swiftly under the reducing conditions of these systems. The TsDPEN ligand plays a critical role in the generation and formatting of the active catalyst including wreaking chiral properties to the so formed catalytic nanoparticles. Kinetic measurements, NMR, UV-visible spectroscopy, circular dichroism (CD) and TEM analyses corroborate this argument." @default.
• W1966282730 created "2016-06-24" @default.
• W1966282730 creator A5048066087 @default.
• W1966282730 creator A5052810976 @default.
• W1966282730 creator A5074812202 @default.
• W1966282730 date "2014-01-01" @default.
• W1966282730 modified "2023-09-28" @default.
• W1966282730 title "The Nature of the True Catalyst in Transfer Hydrogenation with Alcohol Donors Using (arene)&lt;sub&gt;2&lt;/sub&gt;Ru&lt;sub&gt;2&lt;/sub&gt;Cl&lt;sub&gt;4&lt;/sub&gt;(II)/TsDPEN Precursor" @default.
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• W1966282730 doi "https://doi.org/10.4236/mrc.2014.33010" @default.
• W1966282730 hasPublicationYear "2014" @default.
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