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- W1966312089 abstract "Mass spectrometry based experiments show that the m/z 46 ion generated in chemical ionization experiments of CO with a trace of water is not the previously proposed formic acid ion, HC(O)OH+ (1). Instead, the more stable dihydroxycarbene ion, HO–C–OH+ (2) is formed. A mechanistic analysis using the CBS-QB3 model chemistry supports the reaction sequence: (CO)2+ + H2O → H2O–CO+ (3), followed by the CO catalyzed isomerization: 3 + CO → 2 + CO. Solitary ions 1 and 2 do not interconvert, but theory and experiment agree that CO also efficiently catalyzes the conversion 1 → 2." @default.
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- W1966312089 date "2004-05-01" @default.
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- W1966312089 title "The isomerization of [H2O–CO]+ and [HC(O)OH]+ into [HO–C–OH]+: proton-transport catalysis by CO" @default.
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- W1966312089 doi "https://doi.org/10.1016/j.cplett.2004.04.014" @default.
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