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- W1966320055 abstract "The development of a discharge oxygen iodine laser (DOIL) requires efficient production of singlet delta oxygen O 2 (α 1 Δ) in electric discharge. It is important to understand the mechanisms of of O 2 α 1 Δ) quenching in these devices. To gain understanding of this mechanisms quenching of O 2 (α ]1 Δ)in O/O 2 /O 3 /CO 2 /He mixtures has been investigated. Oxygen atoms and singlet oxygen molecules were produced by the 248 nm laser photolysis of ozone. The kinetics of O 2 (α 1 Δ) quenching were followed by observing the 1268 nm fluorescence of O 2 α 1 Δ → X 3 Σ transition. It is shown that vibrationally excited ozone O 3 (υ;) formed in the three-body recombination O + O 2 + M →O 3 (υ) + M is an important O/O 2 /O 3 quenching agent in O/O 2 /O 3 systems. The process O 3 (υ ≥2) + O 2 ( a 1 Δ)→ 2O 2 + O is the main O 2 (α 1 Δ) deactivation channel in the post-discharge zone. If no measures are taken to decrease oxygen atom concentration, the contribution of this process into overall O 2 (α 1 Δ) removal is significant even in the discharge zone. It was found in experiment that addition of species that are good quenchers of O 3 (υ;) decrease O 2 ( a 1 Δ) deactivation rate in the O/O 2 /O 3 mixtures." @default.
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- W1966320055 date "2015-02-03" @default.
- W1966320055 modified "2023-09-23" @default.
- W1966320055 title "Molecular singlet delta oxygen quenching kinetics in the EOIL system" @default.
- W1966320055 doi "https://doi.org/10.1117/12.2064825" @default.
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