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• W1966366987 abstract "Only quinones with a 2-methoxy group can act simultaneously as the primary (QA) and secondary (QB) electron acceptors in photosynthetic reaction centers from Rhodobacter sphaeroides. 13C hyperfine sublevel correlation measurements of the 2-methoxy in the semiquinone states, SQA and SQB, were compared with quantum mechanics calculations of the 13C couplings as a function of the dihedral angle. X-ray structures support dihedral angle assignments corresponding to a redox potential gap (ΔEm) between QA and QB of ∼180 mV. This is consistent with the failure of a ubiquinone analogue lacking the 2-methoxy to function as QB in mutant reaction centers with a ΔEm of ≈160–195 mV." @default.
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• W1966366987 date "2013-10-02" @default.
• W1966366987 modified "2023-09-27" @default.
• W1966366987 title "Tuning Cofactor Redox Potentials: The 2-Methoxy Dihedral Angle Generates a Redox Potential Difference of >160 mV between the Primary (Q_A) and Secondary (Q_B) Quinones of the Bacterial Photosynthetic Reaction Center" @default.
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• W1966366987 doi "https://doi.org/10.1021/bi4011896" @default.
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