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- W1966377615 abstract "A two‐dimensional model is developed to approach the spectral properties of a diatomic polar molecule embedded in a monatomic crystal. This model introduces two rotational degrees of freedom in the limit of small amplitude oscillations. The first one describes the angular (planar) motion of the dipole moment of the molecule. The second one is connected to some collective motion of the nearest atom neighbors of this molecule (called the first shell). The remaining atoms of the crystal act as a thermal bath. This problem is treated first in a classical and then in a quantum version. The experimental data presently available (i.e., for CO molecules trapped in argon crystal) are compared to the theoretical results." @default.
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- W1966377615 date "1982-02-15" @default.
- W1966377615 modified "2023-10-17" @default.
- W1966377615 title "A two‐dimensional model for the infrared and microwave spectrum of diatomic molecules trapped in monatomic crystals" @default.
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- W1966377615 doi "https://doi.org/10.1063/1.443199" @default.
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