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- W1966455770 abstract "A crystalline porous metal–organic framework Cu2(BPDC)2(BPY) was synthesized and characterized by X-ray powder diffraction (XRD), scanning electron microscopy (SEM), transmission electron microscopy (TEM), thermogravimetric analysis (TGA), Fourier transform infrared (FT-IR) spectra, atomic absorption spectrophotometry (AAS), hydrogen temperature-programmed reduction (H2-TPR), and nitrogen physisorption measurements. The Cu-MOF could be used as an efficient heterogeneous catalyst for the copper-catalyzed cross-dehydrogenative coupling reaction of ethers with 2-carbonyl-substituted phenols. The Cu2(BPDC)2(BPY) exhibited significantly higher catalytic activity than that of other Cu-MOFs such as Cu3(BTC)2, Cu(BDC), and Cu(BPDC). The Cu-MOF also offered advantages over several copper salts such as CuCl2, CuCl, CuI, Cu(NO3)2, and Cu(OAc)2 in terms of the catalytic activity as well as the catalyst reusability. To the best of our knowledge, the cross-dehydrogenative coupling reaction of ethers with 2-carbonyl-substituted phenols via C–H activation under oxidative conditions using a heterogeneous catalyst was not previously mentioned in the literature." @default.
- W1966455770 created "2016-06-24" @default.
- W1966455770 creator A5061799227 @default.
- W1966455770 creator A5065826659 @default.
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- W1966455770 date "2013-10-01" @default.
- W1966455770 modified "2023-10-16" @default.
- W1966455770 title "Expanding applications of copper-based metal–organic frameworks in catalysis: Oxidative C–O coupling by direct C–H activation of ethers over Cu2(BPDC)2(BPY) as an efficient heterogeneous catalyst" @default.
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- W1966455770 doi "https://doi.org/10.1016/j.jcat.2013.06.006" @default.
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