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- W1966514059 abstract "New η5-cyclopentadienyl-η1-amido monoalkyl zirconium compounds of the type [ZrR(η5-C5H4SiMe2-η1-NtBu)(η5-C5H4R′)] (R = Me, Bn; R′ = H, SiMe3, SiMe2CH2CH═CH2) have been synthesized and fully characterized. Allyldimethylsilylcyclopentadienyl derivatives [ZrR(η5-C5H4SiMe2-η1-NtBu)(η5-C5H4SiMe2CH2CH═CH2)] isomerize the allyl fragment bound to the cyclopentadienyl ring to give the corresponding [ZrR(η5-C5H4SiMe2-η1-NtBu)(η5-C5H4SiMe2CH═CHCH3)] compounds (R = Me, Bn). Experimental as well as DFT computational studies support an isomerization mechanism based on a N-assisted 1,3-proton shift." @default.
- W1966514059 created "2016-06-24" @default.
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- W1966514059 date "2009-06-16" @default.
- W1966514059 modified "2023-09-23" @default.
- W1966514059 title "Amidosilylcyclopentadienyl Monoalkyl Zirconium Compounds: Evidence of a N-Assisted 1,3-Proton Shift Olefin Isomerization Mechanism" @default.
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- W1966514059 doi "https://doi.org/10.1021/om900296a" @default.
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