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• W1966598634 endingPage "8050" @default.
• W1966598634 startingPage "8042" @default.
• W1966598634 abstract "The conformational properties of 1-bromo-2-chloroethane (BCE) in several representative zeolites including silicalite-1, siliceous Y (Si-Y), Na-Y, and zeolite L have been investigated by FT-Raman spectroscopy in combination with thermogravimetric analysis. The results indicate that the conformational and dynamic behavior of BCE inside a zeoltic host is strongly influenced by several factors such as the framework topology, the Si/Al ratio, and the nature and the locations of charge-balancing cations. For siliceous zeolites (silicalite-1 and Si-Y), the anti population of BCE increases significantly relative to pure liquid upon initial loading at room temperature. Interestingly, when lowering temperature, the anti population of BCE in silicalite-1 continues to increase, but the conformational equilibrium of BCE inside Si-Y shifts to the gauche conformer. Zeolite L and Na-Y with extra-framework cations show an almost exclusive preference for the gauche mode of the BCE molecule at room temperature, and the conformational population does not change significantly at low temperatures." @default.
• W1966598634 created "2016-06-24" @default.
• W1966598634 creator A5008557264 @default.
• W1966598634 creator A5022728200 @default.
• W1966598634 date "2009-04-17" @default.
• W1966598634 modified "2023-09-24" @default.
• W1966598634 title "A Conformational Study of 1-Bromo-2-chloroethane in Zeolites" @default.
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• W1966598634 doi "https://doi.org/10.1021/la9002675" @default.
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