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• W1966736073 startingPage "2317" @default.
• W1966736073 abstract "The equilibrium between excited iodine atoms and oxygen has been examined by monitoring the time‐dependent I*[≡I(2P1/2)] concentration following creation of this species by pulsed laser photolysis of iodine‐containing precursors. A double exponential decay is observed which reflects a fast approach to equilibrium followed by a slower relaxation of the equilibrated mixture. Data obtained with the I* precursors HI and CH3I show that the rate constant for the reaction I*+O2→I+O2 is insignificant compared to that for the reaction I*+O2→I+O2(1Δ). Data obtained from the precursors i‐C3F7I, n‐C3F7I, C2H5I, and CF3I suggest that O2(1Δ) is rapidly relaxed by the precursor itself, by the precursor radical, or by some product formed in a reaction between the precursor radical and oxygen. The rate constant for the process I*+O2→I+O2(1Δ) has been found to be (8.8±0.9)×105 s−1 Torr−1, while that for the process I*+O2→I+O2 is (0.3±1.3)×105 s−1 Torr−1." @default.
• W1966736073 created "2016-06-24" @default.
• W1966736073 creator A5023296050 @default.
• W1966736073 creator A5085840608 @default.
• W1966736073 date "1983-03-01" @default.
• W1966736073 modified "2023-10-18" @default.
• W1966736073 title "The I(²<i>P</i>_1/2)+O₂⇄I(²<i>P</i>_3/2)+O₂(¹Δ) equilibrium" @default.
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• W1966736073 doi "https://doi.org/10.1063/1.445085" @default.
• W1966736073 hasPublicationYear "1983" @default.
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