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- W1966746772 abstract "We developed time-domain ab initio simulation of Auger phenomena, including multiple exciton generation (MEG) and recombination (MER). It is the first approach describing phonon-assisted processes and early dynamics. MEG starts below the electronic threshold, strongly accelerating with energy. Ligands are particularly important to phonon-assisted MEG, which therefore can be probed with infrared spectroscopy. Short-time Gaussian component gives 5−10% of MEG, justifying rate theories that assume exponential dynamics. MER is preceded by electron−phonon relaxation to low energies." @default.
- W1966746772 created "2016-06-24" @default.
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- W1966746772 date "2011-03-31" @default.
- W1966746772 modified "2023-10-01" @default.
- W1966746772 title "Time-Domain ab Initio Study of Auger and Phonon-Assisted Auger Processes in a Semiconductor Quantum Dot" @default.
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- W1966746772 doi "https://doi.org/10.1021/nl200651p" @default.
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