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• W1966771203 abstract "Rotational relaxation kinetics in gas mixtures is calculated by non-Markovian binary theory methods and by means of Anderson—Talman theory which takes into account the multiparticle interaction of the molecule with independently moving buffer atoms. The latter model is the only one which yields a rigorous solution of the problem for any density of atoms. Both approaches are compared in order to check the validity of the binary approximation and to discriminate between the differential and integral formalisms. The program is implemented within the framework of the simplest model of J-diffusion which adequately reproduces the asymptotic behavior of the rotational relaxation for short and long times. The accuracy of the binary theory is ascertained and the appearance of sign-alternating behavior of the correlation function at high densities is shown to be illusive at least in this model." @default.
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• W1966771203 date "1992-07-01" @default.
• W1966771203 modified "2023-10-16" @default.
• W1966771203 title "The angular momentum relaxation due to multiparticle collisions of molecules with atoms" @default.
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• W1966771203 doi "https://doi.org/10.1016/0301-0104(92)87128-v" @default.
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