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• W1966771885 endingPage "143" @default.
• W1966771885 startingPage "133" @default.
• W1966771885 abstract "The use of ‘cation-like’ metallocene combination catalysts (Cp′2MCl22BuLiB(C6F5)3; Cp′ = η5-cyclopentadienyl, or substituted η5-cyclopentadienyl; M = Ti, Zr, Hf, U) for dehydropolymerization of silanes significantly improves the polymer molecular weight. For example, under the same conditions a Cp(C5Me5)ZrCl22BuLi catalyst gives Mn = 1890, while a Cp(C5Me5)ZrCl22BuLiB(C6F5)3 gives Mn = 7270. The influence of various factors (steric and electronic effects of the cyclopentadienyl ligands, the nature of the metal, temperature, solvent, concentration and structure of silane) on the build-up of polysilane chains are systematically analyzed." @default.
• W1966771885 created "2016-06-24" @default.
• W1966771885 creator A5006117349 @default.
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• W1966771885 date "1996-08-01" @default.
• W1966771885 modified "2023-09-27" @default.
• W1966771885 title "A systematic analysis of the structure-reactivity trends for some ‘cation-like’ early transition metal catalysts for dehydropolymerization of silanes" @default.
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• W1966771885 doi "https://doi.org/10.1016/0022-328x(96)06357-7" @default.
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