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- W1966992059 abstract "CO2 in the air can be efficiently captured with simultaneous activation by PEI (polyethyleneimine) to form ammonium carbamate and/or carbonate species. Thus, the in situ hydrogenation of captured CO2 into energy-storage materials rather than going through the desorption of conventional CCS (carbon capture and storage) runs better in comparison with equivalent gaseous CO2, thus validating this potential application of CCU (carbon capture and utilization) for supplying renewable energy. PEI600 as an effective carbon absorbent in this study could also be assumed to serve as both ligand and base to promote the catalytic hydrogenation of captured CO2, consequently acting as a ‘hinge base’ to combine capture and hydrogenation processes. The pathway was studied by NMR and in situ FT-IR spectroscopy under CO2 pressure. This protocol could open up great potential in transforming the captured CO2 from waste to fuel-related products." @default.
- W1966992059 created "2016-06-24" @default.
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- W1966992059 date "2013-01-01" @default.
- W1966992059 modified "2023-10-16" @default.
- W1966992059 title "In situ hydrogenation of captured CO2 to formate with polyethyleneimine and Rh/monophosphine system" @default.
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- W1966992059 doi "https://doi.org/10.1039/c3gc41265b" @default.
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