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• W1967196642 abstract "The methods of steady-state and pulsed millimeter-wave rotational spectroscopy were used to probe the vibrationally excited products, CS and SO produced in the laser photolysis of CS2 and SO2 at 193 nm. The time dependence of the vibrational populations was measured for CS up to v=8 and for SO up to v=5. For CS, a Boltzmann-like population distribution was found with a vibrational temperature of 5795 K corresponding to a vibrational energy of 9.8 kcal mol−1. In the case of SO, significant excitation was observed only for the states v=0, 1 and 2 with v=2 having the largest initial population. A small percentage of the SO molecules were found in v=5. The precursor gases were diluted in Ar to enhance the ratio of rotational to vibrational relaxation times. Because rotational transitions were probed, it was necessary to wait for rotational equilibrium to be established before making the measurements. As a result, the vibrational populations may have been partially relaxed at the time of measurement. In order to evaluate the extent of relaxation, a discussion of the various relaxation processes is given." @default.
• W1967196642 created "2016-06-24" @default.
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• W1967196642 date "1986-12-15" @default.
• W1967196642 modified "2023-09-26" @default.
• W1967196642 title "Millimeter-wave observations of vibrationally excited SO and CS produced by laser photolysis" @default.
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• W1967196642 doi "https://doi.org/10.1063/1.451398" @default.
• W1967196642 hasPublicationYear "1986" @default.
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