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• W1967589029 abstract "A series of binuclear ruthenium(II)−bis(2,2‘:6‘,2‘ ‘-terpyridine) complexes has been prepared around a central biphenylene unit equipped with a strap of variable length. Partial oxidation forms the mixed-valence complex that displays both ligand-to-metal, charge-transfer, and intervalence charge-transfer (IVCT) transitions in the near-IR region. On the basis of Hush theory, the electronic coupling matrix element for interaction between the metal centers decreases with increasing length of the tethering strap. This effect arises because the strap modulates the torsion angle between the phenyl rings and thereby controls the extent of through-bond electronic coupling. The coupling element favors a maximum for planar geometries and a minimum for orthogonal structures, but the full impact of the torsion angle is not realized due to thermal fluctuations." @default.
• W1967589029 created "2016-06-24" @default.
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• W1967589029 date "2004-10-01" @default.
• W1967589029 modified "2023-09-23" @default.
• W1967589029 title "Orientational Control of Electronic Coupling in Mixed-Valence, Binuclear Ruthenium(II)−Bis(2,2‘:6‘,2‘ ‘-Terpyridine) Complexes" @default.
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• W1967589029 doi "https://doi.org/10.1021/ja0451968" @default.
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