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• W1967630555 endingPage "035101" @default.
• W1967630555 startingPage "035101" @default.
• W1967630555 abstract "Ab initio-based configuration interaction studies on RbHe and He–Rb–He have explored some key features of the low-lying electronic states of these van der Waals systems. The radiative lifetime of the Rb*He exciplex has been calculated to be around 24.5 ns, which is slightly higher than the HeRb*He lifetime (∼20 ns) and lower than the atomic fluorescence lifetime of Rb, by roughly 3.5 ns. Better exciplex stability of the symmetric triatomic system is evidenced by its higher binding energy value in comparison to the diatomic system by a substantial margin. BSSE-corrected spin–orbit calculations of RbHe have predicted a potential barrier of the 12Π1/2 state with a height of 15 cm−1 and width of 2.57 Å. The 2Πu state of the triatomic molecule shows a conical intersection of its Renner–Teller components (12A1 and 12B2) near a 99° bond angle along the bending path. Their unstable higher excited states (12Σ+1/2 or 12Σ+g,1/2) can trigger the pumping of the blue side of the ns2S1/2 → np2P3/2 transition, and this may eventually lead to the np2P1/2 →ns2S1/2 lasing transition. The broad fluorescence band with a peak near 11 900 cm−1 is found to arise from the 12Π3/2–X2Σ+1/2 transition of RbHe." @default.
• W1967630555 created "2016-06-24" @default.
• W1967630555 creator A5006616357 @default.
• W1967630555 date "2012-01-11" @default.
• W1967630555 modified "2023-09-26" @default.
• W1967630555 title "Spectroscopic properties of the low-lying electronic states of RbHe<i>_n</i>(<i>n</i>= 1, 2) and their comparison with lighter alkali metal-helium systems" @default.
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• W1967630555 doi "https://doi.org/10.1088/0953-4075/45/3/035101" @default.
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