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• W1968058309 endingPage "1889" @default.
• W1968058309 startingPage "1872" @default.
• W1968058309 abstract "The electrical mobilities of multiply-charged nanodrops of the ionic liquid 1-ethyl, 3-methylimidazolium dicyanamide (EMI-N[CN]2) were accurately measured in air at 20 °C for mass-selected clusters of composition [EMI-N[CN]2]n[EMI+]z, with 2 ≤ n ≤ 369 and 1 ≤ z ≤ 10. We confirm prior reports that the mobility Z of a globular ion of mass m is given approximately by the modified Stokes–Millikan law for spheres, Z = ZSM,mod(dm + dg, z, m), where dm = (6m/πρ)1/3 is the nanodrop mass-diameter based on the density ρ of the liquid (corrected for the capillary compression and electrostatic deformation of the nanodrop), and dg is an effective air molecule diameter. There is however a measurable (up to 7 %) and systematic z-dependent departure of Z from ZSM,mod. As theoretically expected at small ε*, this effect is accurately described by a simple correction factor of the form Z/ZSM,mod = δ(1 − βε*), where kTε* is the potential energy due to the ion–induced dipole (polarization) attraction between a perfectly-conducting charged nanodrop and a polarized neutral gas-molecule at a distance (dm + dg)/2 from its center. An excellent fit of this model to hundreds of data points is found for dg ≈ 0.26 nm, β ≈ 0.36, and δ ≈ 0.954. Accounting for the effect of polarization decreases dg considerably with respect to values inferred from earlier nanodrop measurements that ignored this effect. In addition, and in spite of ambiguities in the mobility calibration scale, the measured constant δ smaller than unity increases Millikan’s drag enhancement factor from the accepted value ξm ≈ 1.36 to the new value ξ ≈ ξm/δ ≈ 1.42 ± 0.03." @default.
• W1968058309 created "2016-06-24" @default.
• W1968058309 creator A5083401528 @default.
• W1968058309 creator A5086452247 @default.
• W1968058309 date "2013-09-19" @default.
• W1968058309 modified "2023-09-25" @default.
• W1968058309 title "Measuring the Effect of Ion-Induced Drift-Gas Polarization on the Electrical Mobilities of Multiply-Charged Ionic Liquid Nanodrops in Air" @default.
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• W1968058309 doi "https://doi.org/10.1007/s13361-013-0702-1" @default.
• W1968058309 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/24048890" @default.
• W1968058309 hasPublicationYear "2013" @default.
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