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- W1968088472 abstract "We apply a previously developed semiclassical complex time method to the calculation of tunneling ionization of several diatomic molecules and CO${}_{2}$. We investigate the presence or absence of the molecular suppression effect by calculating ionization rates of ${mathrm{N}}_{2}$ versus Ar, ${mathrm{O}}_{2}$ versus Xe, ${mathrm{F}}_{2}$ versus Ar, and CO versus Kr. Comparisons with other theories, including the molecular-orbital-Ammosov-Delone-Krainov (MO-ADK) model and the strong-field approximation, are given. We also analyze the dependence of the ionization rate on the angle ${ensuremath{theta}}_{F}$ between the molecular axis and the field direction. The theoretical results agree quite well with experiment for ${mathrm{N}}_{2}$ and ${mathrm{O}}_{2}$ but give too low a value of the peak angle ${ensuremath{theta}}_{F}$ for CO${}_{2}$. Our calculations give small values of the ionization rates for ${mathrm{O}}_{2}$ and CO${}_{2}$ at ${ensuremath{theta}}_{F}=0$ and ${90}^{ifmmode^circelsetextdegreefi{}}$, in agreement with experiment. Other calculations, including the MO-ADK model and methods involving a numerical integration of the time-dependent Schrodinger equation, exhibit substantially weaker suppression at these angles." @default.
- W1968088472 created "2016-06-24" @default.
- W1968088472 creator A5016051232 @default.
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- W1968088472 date "2010-03-22" @default.
- W1968088472 modified "2023-10-16" @default.
- W1968088472 title "Semiclassical complex-time method for tunneling ionization: Molecular suppression and orientational dependence" @default.
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- W1968088472 doi "https://doi.org/10.1103/physreva.81.033417" @default.
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