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- W1968236871 abstract "Two-dimensional arborols are bolaform amphiphiles in which a central, hydrophobic spacer separates twin hydrophilic ends. Under appropriate conditions, these relatively small molecules assemble into very long fibers; subsequently, the system gels if the arborol concentration is sufficiently high. The diffusion of linear or slightly branched dextran probes in 3 and 6% arborol gels, as determined by fluorescence photobleaching recovery, resembles that of dextrans in water, suggesting a highly open network structure. Melting the gels produces almost no change in diffusion of the dextran probes. Small-angle X-ray scattering (SAXS) of wet arborol gels at different concentrations and temperatures reveals the diameter of the repeating unit of the fibers to be 8.26 ± 0.68 nm. This dimension, which is independent of concentration and temperature, exceeds the length of a single arborol molecule by about a factor of 3. Rheological investigation identifies the linear response regime of the gels and permits an examination of the weak correlation between dextran probe diffusion and gel viscoelasticity." @default.
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- W1968236871 date "2007-12-11" @default.
- W1968236871 modified "2023-09-27" @default.
- W1968236871 title "Diffusion of Dextran Probes in a Self-Assembled Fibrous Gel Composed of Two-Dimensional Arborols" @default.
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- W1968236871 doi "https://doi.org/10.1021/jp077050b" @default.
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