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- W1968652470 abstract "Modeling and simulations of compartmentalization effects in tandem with nitroxide exit and entry have been performed for the nitroxide-mediated radical polymerization (NMP) of styrene in an aqueous dispersed system employing 2,2,6,6-tetramethylpiperidinyl-1-oxy (TEMPO) at 125 °C. It is demonstrated that, even for a relatively water-insoluble nitroxide like TEMPO, exit and entry can strongly influence the polymerization kinetics in submicrometer-size droplets/particles. In such systems, the polymerization is expected to proceed at a markedly higher rate than the corresponding bulk system at the expense of control/livingness. Depending on the deactivator water solubility, these findings will apply qualitatively to all controlled/living radical polymerization systems governed by the persistent radical effect [e.g., NMP and atom transfer radical polymerization (ATRP)]." @default.
- W1968652470 created "2016-06-24" @default.
- W1968652470 creator A5017973525 @default.
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- W1968652470 date "2012-05-21" @default.
- W1968652470 modified "2023-09-27" @default.
- W1968652470 title "Synergistic Effects of Compartmentalization and Nitroxide Exit/Entry in Nitroxide-Mediated Radical Polymerization in Dispersed Systems" @default.
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- W1968652470 doi "https://doi.org/10.1021/mz3001786" @default.
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