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- W1968804552 abstract "We discuss to which extent the concepts of Zintl phases and of ‘phonon glasses and electron single crystals’ apply to type-I clathrates. In (β-) Eu8Ga16Ge30 the presence of residual charge carriers appears to be related to a slight off-stoichiometry of the samples pointing to the validity of the Zintl concept in stoichiometric samples. The low and almost stoichiometry independent mobilities of (β-) Eu8Ga16Ge30, Sr8Ga16Ge30, and Ba8Ga16Ge30 seriously question the validity of the ‘electron single crystal’ concept for type-I clathrates. The temperature dependence of the thermal conductivity of a Ba8Ga16Ge30 single crystal indicates that tunneling states play a central role in producing ‘phonon glass’-like thermal conductivities." @default.
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- W1968804552 date "2003-04-01" @default.
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- W1968804552 title "Are type-I clathrates Zintl phases and ‘phonon glasses and electron single crystals’?" @default.
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- W1968804552 doi "https://doi.org/10.1016/s0921-4526(02)01805-7" @default.
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