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- W1968974316 abstract "BaMxAl12−xO19−δ (M = Mn, Fe, Co, x = 1, 2) hexaaluminate nanomaterials were successfully prepared using the ARS (Activated Reactive Synthesis) process, a top-down and solvent free original synthesis route. The crystal sizes of the nanomaterials range at 24 ± 2 nm, which allows them to display high surface area (from 60 to 100 m2 g−1). The role of Mn+ cations in the redox and oxygen transfer properties of the nanomaterials was studied by H2-TPR and 18O/16O isotopic exchange, respectively. The nature of the transition metal as well as its content is observed to play a key role in the oxygen transfer properties. The catalytic properties of the nano-hexaaluminates, evaluated for methane oxidation, a reaction involving severe conditions (high temperature), resulted from multiple factors including oxygen transfer properties and transition metal valence and concentration on the surface." @default.
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- W1968974316 date "2013-01-01" @default.
- W1968974316 modified "2023-10-18" @default.
- W1968974316 title "Role of Mn+ cations in the redox and oxygen transfer properties of BaMxAl12−xO19−δ (M = Mn, Fe, Co) nanomaterials for high temperature methane oxidation" @default.
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- W1968974316 doi "https://doi.org/10.1039/c3cy00192j" @default.
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