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- W1969069585 abstract "Using picosecond CARS the dephasing rate of the ν1-mode of CS2 is investigated in several solvents and in the neat liquid. A large pressure effect (factor of ≤3) is reported for the range 0 to 4 kbar similar to spontaneous Raman results. For an extended interval of 160 to 450 K, a non-monotonic temperature dependence is reported for the first time and compared with theoretical models. — A novel non-degenerate CARS spectrometer is described with 80 fs time resolution and improved measuring accuracy. A dephasing time of T2 = 608 ± 6 fs is reported for the ν1 mode of neat acetone of 293 K; negligible inhomogeneous broadening (< 1%) is indicated by the scattering data for this vibration." @default.
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- W1969069585 date "1990-03-01" @default.
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- W1969069585 title "Vibrational Dephasing of Simple Liquids Investigated by Picosecond and Femtosecond CARS" @default.
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- W1969069585 doi "https://doi.org/10.1002/bbpc.19900940339" @default.
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