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- W1969138524 abstract "New procedures are reported for the specification of caging yields in nuclear recoil chemistry experiments. All five hot 18F substitution channels in CH3CF3 and CH3CHF2 exhibit caging at large density. The respective total caged yields at 195 °K are 4.0%±0.6% and 5.6%±0.6%, and the total yields of stabilized substitution products are 8.9%±0.4% and 8.6%±0.6%. The simplest plausible caging mechanism involves primary Franck–Rabinowitsch radical recombination of 18F atoms with aliphatic radicals. Density-variation results cannot be used for the qualitative detection of caging reactions unless excitation-stabilization complications have been shown to be unimportant." @default.
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- W1969138524 date "1976-06-15" @default.
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- W1969138524 title "Chemistry of nuclear recoil 18F atoms. VIII. Mechanisms and yields of caging reactions in liquid phase 1,1-difluoroethane and 1,1,1-trifluoroethane" @default.
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- W1969138524 doi "https://doi.org/10.1063/1.432133" @default.
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