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- W1969561520 endingPage "9838" @default.
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- W1969561520 abstract "We succeeded in integrating single-wall carbon nanotubes (SWNTs), several water-soluble pyrene derivatives (pyrene-), which bear negatively charged ionic headgroups, and a series of water-soluble metalloporphyrins (MP8+) into functional nanohybrids through a combination of associative van der Waals and electrostatic interactions. The resulting SWNT/pyrene- and SWNT/pyrene-/MP8+ were characterized by spectroscopic and microscopic means and were found to form stable nanohybrid structures in aqueous media. A crucial feature of our SWNT/pyrene- and SWNT/pyrene-/MP8+ is that an efficient exfoliation of the initial bundles brings about isolated nanohybrid structures. When the nanohybrid systems are photoexcited with visible light, a rapid intrahybrid charge separation causes the reduction of the electron-accepting SWNT and, simultaneously, the oxidation of the electron-donating MP8+. Transient absorption measurements confirm that the radical ion pairs are long-lived, with lifetimes in the microsecond range. Particularly beneficial are charge recombination dynamics that are located deep in the Marcus-inverted region. We include, for the first time, work devoted to exploring and testing FeP8+ and CoP8+ in donor−acceptor nanohybrids." @default.
- W1969561520 created "2016-06-24" @default.
- W1969561520 creator A5021721424 @default.
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- W1969561520 creator A5074191348 @default.
- W1969561520 date "2005-06-15" @default.
- W1969561520 modified "2023-10-16" @default.
- W1969561520 title "Functional Single-Wall Carbon Nanotube NanohybridsAssociating SWNTs with Water-Soluble Enzyme Model Systems" @default.
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