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- W1969563185 abstract "A VUV (vacuum-UV) three-photon hot molecule reaction is demonstrated in this study for gaseous triphenylmethane (TPM). A TPM radical was derived from vibrationally hot TPM, which sequentially absorbed the second and third photons within a laser pulse. In the condensed phase, TPM radical was formed by the deprotonation of a cation radical, which was formed by the two-photon ionization. The multiphoton reaction via a hot molecule is a special case which can produce a neutral radical directly. This study also shows that more than two high-energy photons (VUV) can be absorbed and accumulated as vibrational energy. It should be emphasized that an internal conversion is not a useless photophysical process, but a very interesting process for forming an important intermediate in multiphoton laser chemistry." @default.
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- W1969563185 date "2000-10-25" @default.
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- W1969563185 title "Vacuum-UV Three-Photon Chemical Reaction via Vibrationally Hot Molecules: Decomposition of Triphenylmethane" @default.
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- W1969563185 doi "https://doi.org/10.1021/jp003017c" @default.
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