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- W1969714709 abstract "A method for producing electronic-state coherences using either collisionally-aided radiative excitation (or optical collision) or laser-induced collisional energy transfer (or radiative collision) is proposed. Two atoms, $A$ and ${A}^{ensuremath{'}}$, collide in the presence of two pulsed-laser fields having frequencies $ensuremath{Omega}$ and ${ensuremath{Omega}}_{1}$. It is shown that by choosing ${ensuremath{Omega}}_{1}ifmmodepmelsetextpmfi{}ensuremath{Omega}$ such that an energy-conserving transition can occur in the composite $A{A}^{ensuremath{'}}$ system, one can create an electronic-state coherence in the $A$ or ${A}^{ensuremath{'}}$ atoms. The coherence can be produced between states of the same or of opposite parity; if it is between states of opposite parity, coherent emission at frequency ${ensuremath{Omega}}_{1}ifmmodepmelsetextpmfi{}ensuremath{Omega}$ may be generated. The relationship of this work to theories of pressure-induced extra resonances in four-wave mixing is discussed." @default.
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- W1969714709 date "1983-11-01" @default.
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- W1969714709 title "Theory of electronic-state coherences produced in combined laser-field—collisional reactions" @default.
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- W1969714709 doi "https://doi.org/10.1103/physreva.28.2900" @default.
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